Well it is a difference between real resolution and a picture inflated to fill a certain area.
I made a test last year.
Configure to run SHIII in windowed mode.
Then start the Game with 640x480, 800x600, 1024x768, 1280x1024, 1600x 1200, ...
And make a Screenshot of a similar content, thus you can compare the screenshots.
Then open the screenshots and compare them.
My result was that the 1280x1024 is the best quality. And that is the resolution the game was originally made for.
Increasing the resolution makes it larger, that is fine, but not better in quality.
You can your graphic card and your monitor blow up the picture to fill the screen. But you can leave the game resolution at 1280x1024.
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