Can't really pick one, but here's few of my favorites:
- L96A1 Sniper rifle from BF2
- Chainsaw from Doom
- Mp5 in pretty much any game
- Kar 98K from Half-life 1 Day of Defeat
- Suomi M/31 SMG from Finnish Defence Forces addon for ArmA
- And last but not least, FN FAL from ACE addon for ArmA
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